ALF results

Fantastic Spectra and where to find them

The generation of ultra-short light pulses with a good spatial structure is the philosopher’s stone of ultrafast pulse physics. These pulses make it possible to study and modify the properties of matter at time scales unreachable by other procedures.

In recent decades, great strides have been made in the generation of high-quality ultrashort pulses among which post-compression techniques stands out. Post-compression techniques consist of widening the spectrum of a pulse during its propagation thanks to nonlinear effects and then correcting its phase to achieve the shortest possible temporal pulse. The most widely used post-compression technique today is based on the nonlinear propagation of a pulse through a hollow core fiber filled with gas. However, in the last decade, with the rise of new lasers, such as the Yb laser, other post-compression methods that do not have to deal with the restrictions presented by hollow core fibers have gained relevance. One of these new post-compression techniques is the nonlinear propagation in multipass cells.

These multipass cells are cavities formed by two spherical mirrors in which the laser beam is introduced in the cavity off-axis, in such a way that the beam is reflected multiple times forming a hyperboloid before leaving the cell. One of the advantages of these cavities is that we can introduce in them a nonlinear medium through which the beam propagates in nonlinearly during the successive round trips.

Building upon this research, we have theoretically explored a post-compression region in multipass cells that allows the generation of wide spectra with smooth profiles that prevent the pulse from presenting too much structure (pre-pulses or post-pulses) once compressed. In order to accomplish this, we have relied on a particular regime explored already in the 80s known as the enhanced frequency chirp regime, and we have adapted it to multipass cells. In this regime, nonlinear effects and dispersion go hand in hand to widen the spectrum while maintaining a smooth structure that supports a very clean temporal profile. We have optimized the parameters of this region for the case of a multipass cavity filled with argon obtaining pulses whose Fourier limit is compressed more than 10 times with respect to the duration of the initial pulse, but above all maintaining an extremely clean structure, which makes it very useful for a variety of applications.

More information at:

Staels, V. W. Segundo, E. Conejero Jarque, D. Carlson, M. Hemmer, H. C. Kapteyn, M. M. Murnane, y J. San Roman. 2023. «Numerical investigation of gas-filled multipass cells in the enhanced dispersion regime for clean spectral broadening and pulse compression». Opt. Express 31(12):18898-906. doi: 10.1364/OE.481054.
No comments
adminFantastic Spectra and where to find them

Micro-spectrometer

Recently, researchers belonging to ALF, have been working in the development of a miniaturized spectrometer in collaboration with the European Space Agency, the Department of Physics and Swiss Nanoscience Institute (University of Basel), the Department of Chemistry and Applied Biosciences (ETH Zurich), the Swiss Federal Laboratories for Materials Science and Technology (Empa) and the Optics and Photonics Technology Laboratory (Ecole Polytechnique Fédérale de Lausanne, EPFL). The device belongs to the family of ultracompact Fourier Transform spectrometers, and it consist of a LiNbO3 chip in which a monomodal waveguide was fabricated with an optimized design to produce a light flux in the vertical direction. In the upper part of the chip a nano-detector (gold nanowire) was placed perpendicularly to the waveguide, together with a quantum dot HgTe nanolayer. The gold nanowire acts as scattering element, sensing the light confined in the waveguide. The nanolayer creates a photocurrent that can be measured. An external mirror placed at the output of the waveguide enables the creation of a standing wave that is monitorized by the nano-detector. The controlled motion of the mirror produces a spatial swept of the standing wave, thus obtaining the measurement of the confined intensity, from which the spectrum is extracted by Fourier transform.

Scheme of the device

After fabrication, it has been demonstrated the efficient operation with resolution better than 50 cm-1 in the near infrared. The active part of the device has a tiny volume as small as 100 μm×100 μm×100 μm, and it could be integrated in the new generation of ultrasmall satellites.

More information at:  

M. Grotevent et al., “Integrated photodetectors for compact Fourier-transform waveguide spectrometers” Nature Photonics 17, 59 (2023). https://doi.org/10.1038/s41566-022-01088-7

No comments
adminMicro-spectrometer

Announcement of defense of doctoral thesis – Javier Prada-Rodrigo

On June 8th, Javier Prada Rodrigo will present his doctoral thesis entitled “Formation and characterization of surface micro- and nanostructures in polymers and polymeric nanocomposites prepared by irradiation with pulsed nano- and femtosecond lasers” and directed by the doctors D. Pablo Moreno Pedraz and Dª. Esther Rebollar González
 

The defense act will take place at 11:30 a.m. in the Francisco de Vitoria classroom of the Escuelas Mayores Building.

No comments
adminAnnouncement of defense of doctoral thesis – Javier Prada-Rodrigo

Announcement of defense of doctoral thesis – Miguel López Ripa

On May 26, Miguel López Ripa will present his doctoral thesis entitled “Development of ultra-stable characterization techniques for ultrashort laser beams” and directed by doctors D. Íñigo Juan Sola Larrañaga and Mr. Benjamin Alonso Fernandez.

The defense act will take place at 10:30 a.m. in the Francisco de Vitoria classroom of the Escuelas Mayores Building.

No comments
adminAnnouncement of defense of doctoral thesis – Miguel López Ripa

Lasers and nanostructured polymers and compounds: influence of properties and parameters

A study of the formation of Laser Induced Periodic Surface Structures (LIPSS) using near-infrared femtosecond pulsed laser irradiation on poly(ethylene terephthalate) (PET) films deposited over gold substrates has been carried out. We report the influence of the gold substrate roughness and the PET film thickness on LIPSS formation and analyze it in terms of the features of the electric field distribution obtained by computer simulations using COMSOLTM. We obtain LIPSS with periods close to the irradiation wavelength as long as the aforementioned substrate and film parameters remain below certain threshold values, in particular for polymer thicknesses below 200 nm and substrate roughness of few nm. However, experiments show the impossibility of LIPSS formation for rough substrates as well as thick films above these threshold values. In our numerical simulations, we notice the generation of Surface Plasmon Polariton (SPP) in the film-substrate interface that gives rise to a periodical field pattern on the surface of the thin film. This periodicity is broken for a certain level of substrate roughness or film thickness. Moreover, the evolution of the period of the SPP as the substrate roughness and film thickness change for given laser parameters is qualitatively in good agreement with the experimental LIPSS period (below but close to the irradiation laser wavelength). In conclusion, the experimental findings are explained by the formation and behavior of SPP in the thin film-substrate interface. On these grounds, we propose that, for our case of study, this SPP formation and the subsequent inhomogeneous rise in temperature induced by the periodic field on the surface of the sample is the leading mechanism contributing to LIPSS formation.

More information at:  

Prada-Rodrigo, J., Rodríguez-Beltrán, R. I., Ezquerra, T. A., Moreno, P., & Rebollar, E. (2023). Influence of film thickness and substrate roughness on the formation of laser induced periodic surface structures in poly(ethylene terephthalate) films deposited over gold substrates. Optics & Laser Technology, 159, 109007. https://doi.org/10.1016/j.optlastec.2022.109007
No comments
adminLasers and nanostructured polymers and compounds: influence of properties and parameters

Use of ultrashort laser pulses as a standard for fracture resistance testing

The use of fracture mechanics for rationalizing the fracture behavior of cemented carbides is valid, as far as sharp cracks, free of residual stresses and subjected to a well-defined stress state are used for assessing fracture toughness. However, machining a very sharp notch on the surface of hardmetals for fracture toughness testing has been a critical issue during many years. Within this context, introduction of surface “through-thickness” _micronotches (SEμVNB) by means of ultrashort pulsed laser ablation (UPLA) is here proposed, implemented and analyzed as an innovative precracking-like route within flexural testing procedures for appropiated evaluation of fracture toughness of cemented carbides. UPLA parameters used for introducing the micronotch are optimized in terms of induced damage ahead of the notch tip. For comparison purposes, fracture toughness is also determined by means of flexural testing of previously cracked single-edge notch beams (SENB-Cracked) as well as specimens with V-notch tips sharpened through diamond polishing using a razor blade, and Palmqvist indentation microfracture method. The satisfactory agreement found between values measured using UPLA-micronotched and SENB-Cracked (reference) specimens allows to conclude that flexural testing of SEμVNB samples is a valid methodology for reliable determination of fracture toughness of hardmetals. This is feasible because of the extremely short time of laser-matter interaction. It yields small and somehow controlled damage in front of the notch tip as a result of shock wave propagation during ablation, which translates into effective precracking of SEμVNB specimens

More information at:  

Ortiz-Membrado, L., Liu, C., Prada-Rodrigo, J., Jiménez-Piqué, E., Lin, L. L., Moreno, P., Wang, M. S., & Llanes, L. (2022). Assessment of fracture toughness of cemented carbides by using a shallow notch produced by ultrashort pulsed laser ablation, and a comparative study with tests employing precracked specimens. International Journal of Refractory Metals and Hard Materials, 108, 105949. https://doi.org/10.1016/j.ijrmhm.2022.105949
No comments
adminUse of ultrashort laser pulses as a standard for fracture resistance testing

ALF-USAL researchers participate in the annual meeting of the European Optical Society (EOSAM 2022)

From September 12 to 16, the annual meeting of the European Optical Society (EOSAM 2022) was held in Porto (Portugal). The Laser and Photonics Applications group (ALF – USAL) has participated in this conference presenting some of the most recent results of the research it is currently carrying out.

The works presented were:

  • Marina Fernández Galán, Enrique Conejero Jarque, Julio San Román. Pulse self-compression down to the sub-cycle regime in hollow capillary fibers with decreasing pressure gradients. TOM 8 Non-linear and Quantum Optics – Oral contribution (Abstract).
  • Miguel López Ripa, Iñigo J. Sola, Benjamín Alonso. Ultraestable spatiotemporal characterization of optical vortices in the visible and near infrared. TOM 13 Advances And Applications of Optics and Photonics – Oral contribution (Abstract). 
  • Rodrigo Martín Hernández, Luis Plaja, Carlos Hernández García. Fourier-limited attosecond pulse generation with magnetically pumped high-order harmonic generation. TOM 8 Non-linear and Quantum Optics – Oral contribution (Abstract)
  • Luis Plaja, Ana García Cabrera, Roberto Boyero-García, Óscar Zurrón, Julio San Román, Carlos Hernández García. Multi-beam vortex generation induced by the non-linear optical anisotropy of graphene. TOM 8 Non-linear and Quantum Optics – Poster (Abstract)
  • Victor W. Segundo Staels, Enrique Conejero Jarque, Daniel Carlson, Michaël Hemmer, Henry C. Kapteyn, Margaret M. Murnane, Julio San Román. Supercontinuum generation in the enhanced frequency chirp regime in multipass cells. TOM 8 Non-linear and Quantum Optics – Oral contribution (Abstract)
  • Carlos Hernández García. Novel ultrafast structured EUV/x-ray sources from nonlinear optics. TOM 13 Advances And Applications of Optics and Photonics – Oral contribution (Abstract). 
No comments
adminALF-USAL researchers participate in the annual meeting of the European Optical Society (EOSAM 2022)

It was not everything perfect

 
Nowadays, the high-order harmonic generation process is an extended useful tool for the study of femtosecond dynamics. Nevertheless, there are still many doubts regarding the electron behavior inside different types of mediums.
 
Recent studies in solid targets have revealed new scenarios with extraordinary electronic dynamics compared with atoms or molecules. The process in solids can be explain through a semiclassical point of view using the electron trajectory from the excitation until the recombination with its hole in real space; the so-called perfect recollisions. However, recent studies have confirmed that part of the high-order harmonic emissions comes from trajectories where the electron and hole do not overlap in real space; the so-called imperfect recollisions.
 
In this work, we demonstrate the existence of imperfect recollisions when the medium is a single-layer graphene, and the driving laser pulse is linearly polarized. Graphene, compared to other solids, presents a singular structure band with points where the valence and conduction band are in contact. Our study has a great relevance because until this moment there were studies only with finite-gap solids and huge Berry curvature or using a driving field with elliptical polarization. We truly believe that this work takes a new step in the full understanding of the ultrafast dynamics driven by intense laser pulses in solids.
 

More information at:

Boyero-García, Roberto, Ana García-Cabrera, Oscar Zurrón-Cifuentes, Carlos Hernández-García, y Luis Plaja. «Non-classical high harmonic generation in graphene driven by linearly-polarized laser pulses». Opt. Express 30, n.o 9 (abril de 2022): 15546-55. https://doi.org/10.1364/OE.452201.
No comments
adminIt was not everything perfect

Meeting in Salamanca of the Scientific Advisory Committee of ATTOSTRUCTURA project

Next August will be thirty months since the ATTOSTRUCTURA project began, which means that half of its duration has already elapsed.

For this reason, the first meeting of the project’s scientific advisory committee has been held. The committee, made up of external researchers who are experts in the different fields of the project, has the objective of evaluating the development of the project, the results obtained to date and, if necessary, proposing changes or modifications in the lines of research. In this way, it is intended to ensure that the project achieves the best possible results while maintaining the highest level of excellence.

The members of the scientific advisory committee are:

  • Prof. Jon Marangos (chairman) –  Imperial College (London, UK)
  • Dra. Alicia Palacios – Universidad Autónoma de Madrid (Madrid, Spain)
  • Prof. Misha Ivanov – Instituto Max Born de Óptica No Lineal y Espectroscopía de Pulso Corto en la Asociación de Investigación de Berlín (Berlin, Germany)
  • Catedrático Jamal Berakdar – Instituto de Física, Universidad Martin-Luther (Halle – Wittenberg, Germany)

The meeting, which took place on Friday, July 22, in the Board Room of the Faculty of Sciences, began with an open-door session in which the status of the project and the main results obtained to date were presented. The videos of that session will be available on the project website.

On the occasion of the meeting, Carlos Hernández García (principal investigator of the project) speaks in this video recorded by the audiovisual services of the University of Salamanca, about the project, its objectives and the results obtained.

No comments
adminMeeting in Salamanca of the Scientific Advisory Committee of ATTOSTRUCTURA project

ALF-USAL researchers participate in the XXXVIII Biennial Meeting of the Royal Spanish Society of Physics (Murcia)

From July 11 to 15, the XXXVIII Biennial Meeting of the Royal Spanish Society of Physics was held. The Laser and Photonics Applications group (ALF – USAL) has participated in said biennial, presenting some of the most recent results of the research it is currently carrying out.

The works presented were:

  • Luis Sánchez-Tejerina, Rodrigo Martín-Hernández, Rocío Yanes, Luis Plaja, Luis López-Díaz, Carlos Hernández-García. “Magnetic order excitation by magnetic fields from sub-picosecond structured laser pulses”. S15 Novel frontiers and challenges in magnetism – Oral contribution. (Abstract)
  • Rodrigo Martín-Hernández, Luis Sánchez-Tejerina, Enrique Conejero Jarque, Luis Plaja , Carlos Hernández-García. “Spatial isolation of femtosecond magnetic needles driven by azimuthally-polarized laser beams“, S15 Novel frontiers and challenges in magnetism – Oral contribution. (Abstract). Prize for the best oral contribution in the Symposium “Novel Frontiers and Challenges in Magnetism” awarded by the Spanish chapter of IEEE Magnetics.
  • Miguel López-Ripa, Íñigo J. Sola, Benjamín Alonso. “In-line and ultraestable spatiotemporal characterization of constant and time-varying optical vortices“, S9 Quantum Optics and Nonlinear Optics – Oral contribution (Abstract)
  • V. W. Segundo Staels, E. Conejero Jarque, J. San Roman. Use of gas-filled multipass cells to generate clean supercontinuum spectra“, S9 Quantum Optics and Nonlinear Optics – Oral contribution. (Abstract)
  • Luis Sánchez-Tejerina, Rodrigo Martín-Hernández, Rocío Yanes, Luis Plaja, Luis López-Díaz, Carlos Hernández-García. “Non-linear, purely magnetic magnetization response to femtosecond structured laser pulses“, S9 Quantum Optics and Nonlinear Optics – Oral contribution. (Abstract)
  • Rodrigo Martín-Hernández,Luis Plaja, Carlos Hernández-García. “Magnetically-pumped High Harmonic Generation with circularly polarized driving fields”, S9 Quantum Optics and Nonlinear Optics – Oral contribution. (Abstract)
  • Ana García-Cabrera, Roberto Boyero-García, Óscar Zurrón Cifuentes, Julio San Román, Carlos Hernández-García, Luis Plaja. “Multi-vortex high-harmonic beams from graphene’s anisotropy“, S9 Quantum Optics and Nonlinear Optics – Oral contribution. (Abstract)
  • Alba de las Heras, Alok Kumar Pandey, Julio San Román, Javier Serrano, Luis Plaja. “Extreme-ultraviolet scalar and vectorial vortices with very high topological charge“, S9 Quantum Optics and Nonlinear Optics – Oral contributionl. (Abstract). Winner of the “Young Researchers” contest in the student category.
  • Ignacio Lopez-Quintas, Warein Holgado, Rokas Drevinskas, Peter G. Kazansky, Íñigo J. Sola, Benjamín Alonso. “Collinear optical vortices with tailored topological charge generated by angular momentum transfer“, S9 Quantum Optics and Nonlinear Optics – Poster. (Abstract)
  • Javier Serrano, Carlos Hernández-García. “High-performance simulations of high-order harmonic generation based on artificial intelligence“, S9 Quantum Optics and Nonlinear Optics – Poster. (Abstract)
  • Rosa Ana Pérez-Herrera, Alba de las Heras, María-Baralida Tomás, Beatriz Santamaría, Clara Benedí-García, Ana I. Gómez-Varela, Verónica González-Fernández, Martina Delgado-Pinar. “The future researchers in Optics and Photonics: gender bias in the PhD theses defended in Spain in 2015-2020“, S2 Women in Physics – Oral contribution. (Abstract). 

In addition, Carlos Hernández García participated in the organization of the congress as part of the scientific committee.

No comments
adminALF-USAL researchers participate in the XXXVIII Biennial Meeting of the Royal Spanish Society of Physics (Murcia)